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Teplofizika vysokikh temperatur, 2001, Volume 39, Issue 1, Pages 26–34 (Mi tvt1849)  

This article is cited in 14 scientific papers (total in 14 papers)

Plasma Investigations

Inelastic interaction of an electron with a $\mathrm{C}_{60}$ cluster

A. A. Vostrikov, D. Yu. Dubov, A. A. Agarkov

Institute of Thermophysics, Siberian Division of the Russian Academy of Sciences, Novosibirsk
Abstract: The method of intersecting beams of $\mathrm{C}_{60}$ fullerene clusters and of electrons is used to investigate the production of $\mathrm{C}_{60}^+$ and $\mathrm{C}_{60}^-$ ions and the radiation in the wavelength range from $300$ to $800$ nm for the electron energy $E_e$ ranging from zero to $100$ eV. The absolute values of the ionization and electron-attachment cross sections [$\sigma^+(E_e )$ and $\sigma^-(E_e)$, respectively] are determined. A maximum of $\sigma^+(E_e)$ of 0.53 nm$^2$ is observed at $E_e=52$ eV. For a $\mathrm{C}_{60}$ cluster excited by electron impact, "delayed" ($\sim­150 \mu$s) ionization initiated by collision with the surface and ionization due to thermionic emission (its characteristic time at $E_e=60$ eV is $6\mu$s) is observed. It is found that, for $E_e < 0.4$ eV, the formation of $\mathrm{C}_{60}^-$ is defined by the polarization capture of an $s$-electron ($\sigma^-\sim E^{-1}_e$), and a formula is suggested for determining $\sigma^-(E_e)$. In the region of $E_e$ from $1$ to $6$ eV, the cross section $\sigma^-(E_e)$ shows only slight variations about $\sigma^-(E_e)=0.36\pm 0.03$ nm$^2$. For $E_e>7.5$ eV, $\mathrm{C}_{60}^-$ ions proved to be unstable to electron autodetachment. In the region of intersection of $\mathrm{C}_{60}$ and electron beams, radiation of a quasicontinuous spectrum described by a modified Planck formula for the thermal emission of spherical particles of diameter $d\ll\lambda$ is recorded. For $E_e>47$ eV, the brightness temperature proved to be $3150\pm50$ K. It is found that this radiation is emitted predominantly by hot $\mathrm{C}_{60}^{+*}$ ions produced as a result of thermionic emission from $\mathrm{C}_{60}^*$. The rate of radiation loss of energy by a $\mathrm{C}_{60}^{+*}$ ion and the cross section for the formation of radiating $\mathrm{C}_{60}^{+*}$ ions are found to be, respectively, $5.5\times 105$ eV/s at $T=3150$ K and $2\times10^{-2}$ nm$^2$ at $E_e=60$ eV.
Received: 23.02.2000
English version:
High Temperature, 2001, Volume 39, Issue 1, Pages 22–30
DOI: https://doi.org/10.1023/A:1004158127791
Document Type: Article
UDC: 539.19.541.5
Language: Russian
Citation: A. A. Vostrikov, D. Yu. Dubov, A. A. Agarkov, “Inelastic interaction of an electron with a $\mathrm{C}_{60}$ cluster”, TVT, 39:1 (2001), 26–34; High Temperature, 39:1 (2001), 22–30
Citation in format AMSBIB
\Bibitem{VosDubAga01}
\by A.~A.~Vostrikov, D.~Yu.~Dubov, A.~A.~Agarkov
\paper Inelastic interaction of an electron with a $\mathrm{C}_{60}$ cluster
\jour TVT
\yr 2001
\vol 39
\issue 1
\pages 26--34
\mathnet{http://mi.mathnet.ru/tvt1849}
\transl
\jour High Temperature
\yr 2001
\vol 39
\issue 1
\pages 22--30
\crossref{https://doi.org/10.1023/A:1004158127791}
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  • This publication is cited in the following 14 articles:
    Citing articles in Google Scholar: Russian citations, English citations
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