Abstract:
We study the origin of the boson peak and an associated mechanism for
acoustic-phonon broadening (below the peak) in glasses exhibiting
a high-frequency sound above the peak. The origin is related to the Ioffe–Regel crossover for inelastic (resonant) scattering of
acoustic phonons from harmonic soft-mode vibrations. The broadening mechanism
is due to the resonant interaction of a harmonic soft-mode vibration with
acoustic phonons, which results in the resonant scattering. We find that
the associated width of the phonon is independent of temperature and is
characterized by a power-law frequency dependence with the exponent varying
from ϰ=2 just below the boson peak to ϰ=4 at lower frequencies. The dependences seem to partly agree with some recent experimental data for the glasses under consideration.
Citation:
M. I. Klinger, “Soft-mode related origin of the boson peak and acoustic-phonon broadening in glasses”, TMF, 154:1 (2008), 77–90; Theoret. and Math. Phys., 154:1 (2008), 64–74
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\by M.~I.~Klinger
\paper Soft-mode related origin of the~boson peak and acoustic-phonon broadening in glasses
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\jour Theoret. and Math. Phys.
\yr 2008
\vol 154
\issue 1
\pages 64--74
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Linking options:
https://www.mathnet.ru/eng/tmf6152
https://doi.org/10.4213/tmf6152
https://www.mathnet.ru/eng/tmf/v154/i1/p77
This publication is cited in the following 3 articles:
Lijun Geng, Qiuying Du, Mengxu Li, Baoqi Yin, Zhixun Luo, Jijun Zhao, “The s‐p Nonhybrid Nature Causes Adaptive Superatomic States of Bismuth Clusters”, Chemistry A European J, 29:51 (2023)
Zaccone A., “Relaxation and Vibrational Properties in Metal Alloys and Other Disordered Systems”, J. Phys.-Condes. Matter, 32:20 (2020), 203001
Baggioli M., Cui B., Zaccone A., “Theory of the Phonon Spectrum in Host-Guest Crystalline Solids With Avoided Crossing”, Phys. Rev. B, 100:22 (2019), 220201