A. M. Zheltikov, A. N. Naumov, “High-resolution four-photon spectroscopy with chirped pulses”, Kvantovaya Elektronika, 30:7 (2000), 606–610 [Quantum Electron., 30:7 (2000), 606

Abstract: We propose new schemes of high-resolution coherent four-photon spectroscopy where chirped pulses are employed for the Raman excitation of a nonlinear medium. The use of linearly chirped pulses in coherent anti-Stokes Raman scattering spectroscopy allows the spectra of nonlinear susceptibility to be studied with a terahertz resolution by measuring the intensity of the signal emerging from four-wave mixing as a function of the delay time between the pump pulses. This approach can be also employed for single-pulse spectroscopy of nonlinear susceptibility.

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