Abstract:
A model is proposed for the activation of O2 by methane monooxygenase using a supported binuclear iron complex as a catalytic centre in the presence of Zn as a reducing agent, methylviologen as a mediator, and acetic acid as an effector.
Document Type:
Article
Language: English
Citation:
V. S. Belova, A. M. Khenkin, V. N. Postnov, V. E. Prusakov, A. E. Shilov, M. L. Stepanova, “Oxidation of Alkanes by Dioxygen in the Presence of an Iron Complex immobilized on Modified Silica. Chemical Model of Methane Monooxygenase”, Mendeleev Commun., 2:1 (1992), 7–8
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E. I. Karasevich, V. S. Kulikova, A. E. Shilov, A. A. Shteinman, “Biomimetic alkane oxidation involving metal complexes”, Russian Chem. Reviews, 67:4 (1998), 335–355
Alexander E. Shilov, Georgiy B. Shul'pin, “Activation of C-H Bonds by Metal Complexes”, Chem. Rev., 97:8 (1997), 2879
A. A. Shteinman, “Structure and catalytic mechanism of methane monooxygenase and approaches to its modelling”, Russ Chem Bull, 44:6 (1995), 975
Tracey J. Hall, Justin S.J. Hargreaves, Graham J. Hutchings, Richard W. Joyner, Stuart H. Taylor, “Catalytic synthesis of methanol and formaldehyde by partial oxidation of methane”, Fuel Processing Technology, 42:2-3 (1995), 151
Ferenc Ungváry, “Transition metals in organic synthesis: Hydroformylation, reduction, and oxidation. Annual survey covering the year 1992”, Journal of Organometallic Chemistry, 477:1-2 (1994), 363
Ki-Won Jun, Eun-Kyung Shim, Seong-Bo Kim, Kyu-Wan Lee, Studies in Surface Science and Catalysis, 82, New Developments in Selective Oxidation II, Proceedings of the Second World Congress and Fourth European Workshop Meeting, 1994, 659
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