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Pis'ma v Zhurnal Èksperimental'noi i Teoreticheskoi Fiziki, 2021, Volume 114, Issue 10, Pages 661–668
DOI: https://doi.org/10.31857/S1234567821220079
(Mi jetpl6553)
 

This article is cited in 5 scientific papers (total in 5 papers)

CONDENSED MATTER

Many-electron effects in th $5p$ and $5s$ X-ray photoelectron spectra of ThO$_2$

V. G. Yarzhemskya, Yu. A. Teterinbc, K. I. Maslakovb, A. Yu. Teterinc, K. E. Ivanovc

a Kurnakov Institute of General and Inorganic Chemistry, Russian Academy of Sciences, Moscow, 119991 Russia
b Faculty of Chemistry, Moscow State University, Moscow, 119234 Russia
c National Research Center Kurchatov Institute, Moscow, 123182 Russia
References:
Abstract: The Th $5p$ photoelectron spectrum of the ThO$_2$ oxide exhibits an anomalous spin–orbit splitting, intense satellite, and a poorly observable very strongly broadened Th $5s$ line. The Th $5p$ and Th $5s$ photoelectron spectra are calculated in this work using the configuration interaction and spectral (Green's) function methods in the basis of atomic Hartree–Fock functions. The results are in good agreement with experiment and indicate that the structure of these spectra is determined by interactions of the photoionization-induced $5p^{-1}$ and $5s^{-1}$ states with the $5d^{-2}5f(\varepsilon f)$ and $5p^{-1}5d^{-1}(\varepsilon f)$ satellite states including two holes and one electron in the discrete or continuous spectrum.
Funding agency Grant number
Ministry of Science and Higher Education of the Russian Federation
The work was performed using equipment acquired with the support of the Program of Development of Moscow State University.
Received: 02.08.2021
Revised: 06.10.2021
Accepted: 06.10.2021
English version:
Journal of Experimental and Theoretical Physics Letters, 2021, Volume 114, Issue 10, Pages 609–615
DOI: https://doi.org/10.1134/S0021364021220136
Bibliographic databases:
Document Type: Article
Language: Russian
Citation: V. G. Yarzhemsky, Yu. A. Teterin, K. I. Maslakov, A. Yu. Teterin, K. E. Ivanov, “Many-electron effects in th $5p$ and $5s$ X-ray photoelectron spectra of ThO$_2$”, Pis'ma v Zh. Èksper. Teoret. Fiz., 114:10 (2021), 661–668; JETP Letters, 114:10 (2021), 609–615
Citation in format AMSBIB
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\by V.~G.~Yarzhemsky, Yu.~A.~Teterin, K.~I.~Maslakov, A.~Yu.~Teterin, K.~E.~Ivanov
\paper Many-electron effects in th $5p$ and $5s$ X-ray photoelectron spectra of ThO$_2$
\jour Pis'ma v Zh. \`Eksper. Teoret. Fiz.
\yr 2021
\vol 114
\issue 10
\pages 661--668
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\crossref{https://doi.org/10.31857/S1234567821220079}
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\jour JETP Letters
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\vol 114
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\pages 609--615
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  • This publication is cited in the following 5 articles:
    Citing articles in Google Scholar: Russian citations, English citations
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    Письма в Журнал экспериментальной и теоретической физики Pis'ma v Zhurnal Иksperimental'noi i Teoreticheskoi Fiziki
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    References:18
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