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Pis'ma v Zhurnal Èksperimental'noi i Teoreticheskoi Fiziki, 2021, Volume 114, Issue 5, Pages 311–317
DOI: https://doi.org/10.31857/S1234567821170043
(Mi jetpl6499)
 

This article is cited in 1 scientific paper (total in 1 paper)

CONDENSED MATTER

New aspects of enhancing the graphene capacitance by defects in aqueous electrolytes and ionic liquids

V. A. Kislenkoab, S. V. Pavlovab, M. V. Fedorova, S. A. Kislenkob

a Center for Computational and Data-Intensive Science and Engineering, Skolkovo Institute of Science and Technology, Moscow, 121205 Russia
b Joint Institute for High Temperatures, Russian Academy of Sciences, Moscow, 125412 Russia
Full-text PDF (591 kB) Citations (1)
References:
Abstract: The influence of internal and external defects in graphene on the capacitance of the graphene/electrolyte interface was explored using Density Functional Theory (DFT) calculations. Aqueous solutions and ionic liquids were considered as electrolyte. The results indicate that in aqueous solutions the intrinsic defects, such as mono- and divacancies, enhance the integral capacitance more effectively than external ones, such as nitrogen impurity and oxygen functional groups, used in practice. On the other hand, the strategy of increasing the integral capacitance by creating defects in graphene is ineffective for ionic liquids with an electrochemical window larger than 2 V.
Funding agency Grant number
Ministry of Science and Higher Education of the Russian Federation АААА-А19-119022190058-2
This work was supported by the Ministry of Science and Higher Education of the Russian Federation (theme no. AAAA-A19-119022190058-2, state assignment for the Joint Institute for High Temperatures, Russian Academy of Sciences.
Received: 01.07.2021
Revised: 24.07.2021
Accepted: 25.07.2021
English version:
Journal of Experimental and Theoretical Physics Letters, 2021, Volume 114, Issue 5, Pages 263–268
DOI: https://doi.org/10.1134/S0021364021170021
Bibliographic databases:
Document Type: Article
Language: Russian
Citation: V. A. Kislenko, S. V. Pavlov, M. V. Fedorov, S. A. Kislenko, “New aspects of enhancing the graphene capacitance by defects in aqueous electrolytes and ionic liquids”, Pis'ma v Zh. Èksper. Teoret. Fiz., 114:5 (2021), 311–317; JETP Letters, 114:5 (2021), 263–268
Citation in format AMSBIB
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\paper New aspects of enhancing the graphene capacitance by defects in aqueous electrolytes and ionic liquids
\jour Pis'ma v Zh. \`Eksper. Teoret. Fiz.
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\vol 114
\issue 5
\pages 311--317
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\crossref{https://doi.org/10.31857/S1234567821170043}
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\jour JETP Letters
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\vol 114
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\pages 263--268
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