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This article is cited in 1 scientific paper (total in 1 paper)
CONDENSED MATTER
Formation of an antiferromagnetic metal phase in the electron-doped Sr$_{0.98}$La$_{0.02}$MnO$_3$ oxide according to $^{17}$O NMR data
Z. N. Volkovaa, S. V. Verkhovskiia, A. P. Gerashchenkoa, A. Yu. Germova, K. N. Mikhaleva, A. Yu. Yakubovskiib, E. I. Konsatntinovac, I. A. Leonidovc a Institute of Metal Physics, Ural Branch, Russian Academy of Sciences, Yekaterinburg, Russia
b National Research Center Kurchatov Institute, Moscow, Russia
c Institute of Solid State Chemistry, Ural Branch, Russian Academy of Sciences, Yekaterinburg, Russia
Abstract:
The spin density distribution of itinerant electrons, $n_{eg}$, and their effect on pairwise correlations of localized spins $S(t_{2g})$ of Mn$^{4+}$ ions in cubic Sr$_{1-x}$La$_x$MnO$_3$ antiferromagnet ($x = 0.02$, $T_{\mathrm{N}} = 230$ K, $\mathrm{G}$ type magnetic structure) is studied experimentally by nuclear magnetic resonance on $^{17}$O nuclei. The regions with $n_{eg}>x$, in which the local spin susceptibility of pairs of Mn atoms follows the dependence $\chi\sim(T-\Theta)^{-1}$ with $\Theta = 20(5)$ K, indicating the growth of ferromagnetic spin correlations of neighboring magnetic ions in these domains, are found in the paramagnetic phase. The fraction of Mn-O-Mn bonds ($n_{eg}>x$) increases with the decrease in the temperature. The interpenetrating meshes of Mn-O-Mn bonds with different densities of itinerant $e_g$ electrons form an antiferromagnetic metal phase below $T_{\mathrm{N}}$. The role of weak localization effects is discussed as the main origin of the magnetic inhomogeneity of the antiferromagnetic metal phase in Sr$_{0.98}$La$_{0.02}$MnO$_3$.
Received: 10.01.2019 Revised: 05.03.2019 Accepted: 07.03.2019
Citation:
Z. N. Volkova, S. V. Verkhovskii, A. P. Gerashchenko, A. Yu. Germov, K. N. Mikhalev, A. Yu. Yakubovskii, E. I. Konsatntinova, I. A. Leonidov, “Formation of an antiferromagnetic metal phase in the electron-doped Sr$_{0.98}$La$_{0.02}$MnO$_3$ oxide according to $^{17}$O NMR data”, Pis'ma v Zh. Èksper. Teoret. Fiz., 109:8 (2019), 552–556; JETP Letters, 109:8 (2019), 541–545
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https://www.mathnet.ru/eng/jetpl5882 https://www.mathnet.ru/eng/jetpl/v109/i8/p552
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