Abstract:
Thin films of MnxSi1−x (x≈0.5) alloy were synthesized by pulsed laser deposition in a droplet-free mode on sapphire substrates with different crystallographic cut-off plane orientations (c-Al2O3 and r-Al2O3) at various laser energy densities E at the polycrystalline target MnSi. X-ray structure properties, as well as static and resonance magnetic characteristics of the films depending on the value of E and substrate orientation were investigated. The presence of a ferromagnetic phase with an unusually high Curie temperature TC∼ 300 K which is untypical of MnSi single crystals (TC≈ 30 K) was revealed in films deposited using high laser energy densities E>6 J/cm2 at the target. The magnetic moment of the films on c-Al2O3 substrates is somewhat larger than in the case of r-Al2O3 substrates. Moreover, the films deposited on c-Al2O3 substrates show significantly higher values of the effective magnetic anisotropy field 4πMeff, measured by ferromagnetic resonance. Obtained data show that the structure of the substrate has a remarkable influence on the formation process and magnetic properties of the high-temperature ferromagnetic phase in the MnxSi1−x films.
Keywords:
MnxSi1−x alloys, pulsed laser deposition, ferromagnetic films, magnetic anisotropy.
The work was supported by the Ministry of Science and Higher Education within the State assignment of the Federal Scientific Research Center “Crystallography and Photonics”, Russian Academy of Sciences in part of "Laser synthesis of MnxSi1−x thin films", and by the Russian Foundation for Basic Research, project nos. 19-29-03032, 19‑07-00471, 19-07-00738, in part of “Investigation of magnetic properties of MnxSi1−x thin films". Low-temperature FMR studies of the films were conducted under the auspices of the Program of fundamental research of the Presidium of the Russian Academy of Sciences “Actual problems of low-temperature physics”.
Citation:
A. B. Drovosekov, L. S. Parshina, O. D. Khramova, D. S. Gusev, O. A. Novodvorskii, A. N. Taldenkov, K. Yu. Chernoglazov, V. V. Ryl'kov, “Influence of substrate crystal structure on the magnetic anisotropy of MnxSi1−x (x≈0.5) films”, Fizika Tverdogo Tela, 63:10 (2021), 1527–1531; Phys. Solid State, 63:11 (2021), 1638–1642
\Bibitem{DroParKhr21}
\by A.~B.~Drovosekov, L.~S.~Parshina, O.~D.~Khramova, D.~S.~Gusev, O.~A.~Novodvorskii, A.~N.~Taldenkov, K.~Yu.~Chernoglazov, V.~V.~Ryl'kov
\paper Influence of substrate crystal structure on the magnetic anisotropy of Mn$_{x}$Si$_{1-x}$ ($x\approx0.5$) films
\jour Fizika Tverdogo Tela
\yr 2021
\vol 63
\issue 10
\pages 1527--1531
\mathnet{http://mi.mathnet.ru/ftt7987}
\crossref{https://doi.org/10.21883/FTT.2021.10.51400.121}
\elib{https://elibrary.ru/item.asp?id=46598569}
\transl
\jour Phys. Solid State
\yr 2021
\vol 63
\issue 11
\pages 1638--1642
\crossref{https://doi.org/10.1134/S1063783421100103}
Linking options:
https://www.mathnet.ru/eng/ftt7987
https://www.mathnet.ru/eng/ftt/v63/i10/p1527
This publication is cited in the following 2 articles:
S. Jena, R. Urkude, W.-Y. Choi, K. K. Pandey, S. Karwal, M. H. Jung, J. Gardner, B. Ghosh, V. R. Singh, “Electronic structures of skyrmionic polycrystalline MnSi thin film studied by resonance photoemission and x-ray near edge spectroscopy”, Journal of Applied Physics, 135:16 (2024)
S. Jena, R. Dawn, W.-Y. Choi, Y. Singh, A. Ghosh, S.K. Sahoo, M.H. Jung, J. Gardner, V.K. Verma, K. Amemiya, V.R. Singh, “Texture, electronic and magnetic states of Mn atoms in polycrystalline MnSi thin films facing a c-sapphire substrate studied by soft X-ray magnetic circular dichroism”, Thin Solid Films, 786 (2023), 140097