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Fizika Goreniya i Vzryva, 2020, Volume 56, Issue 3, Pages 61–68
DOI: https://doi.org/10.15372/FGV20200306 (Mi fgv679) 		 
This article is cited in 4 scientific papers (total in 4 papers)

Thermochemical and energy characteristics of symmetric nitro and azido derivatives of diazen-ter-furazanes

D. B. Lemperta, A. I. Kazakova, V. S. Sannikovb, A. V. Nabatovaa, D. V. Dashkob, A. I. Stepanovb

a Institute of Problems of Chemical Physics, Russian Academy of Sciences, 142432, Chernogolovka, Russia
b Tekhnolog Special Design and Technological Bureau, 193076, St. Petersburg, Russia
Full-text PDF (228 kB) Citations (4)
DOI: https://doi.org/10.15372/FGV20200306
Abstract: The heat of combustion and enthalpy of formation of bis(4"-nitro[3,3':4',3"]terfurazan-4-yl)-diazene (DNFNF) and (bis(4"-azido-[3,3':4',3"]terfurazan-4-yl)-diazene (DAzFNF) were first experimentally determined. It is found that the energy increment of the substitution of the azide group for the nitro group in the furazan cycle averages 290 kJ/mol and is close to the increment of substitution of $\mathrm{N}_3$ for $\mathrm{NO}_2$ in trinitroethane. The dependence of the energy parameters of metal-free rocket propellants based on a mixture of ammonium perchlorate with DNFNF or with DAzFNF with an active binder on the content of the highly enthalpy component in the formulation was studied by thermodynamic analysis.
Keywords: bis(4"-nitro[3,3':4',3"]terfurazan-4-yl)-diazene, bis(4"-azido-[3,3':4',3"]terfurazan-4-yl)-diazene, enthalpy of combustion, enthalpy of formation, partial contribution, solid composite propellant (SCP), specific impulse.
Funding agency Grant number
Ministry of Science and Higher Education of the Russian Federation 0089-2014-0019
Received: 08.04.2019
Revised: 14.06.2019
Accepted: 28.08.2019
English version:
Combustion, Explosion and Shock Waves, 2020, Volume 56, Issue 3, Pages 301–307
DOI: https://doi.org/10.1134/S0010508220030065
Bibliographic databases:
Document Type: Article
UDC: 541.11:547.235.5
Language: Russian
Citation: D. B. Lempert, A. I. Kazakov, V. S. Sannikov, A. V. Nabatova, D. V. Dashko, A. I. Stepanov, “Thermochemical and energy characteristics of symmetric nitro and azido derivatives of diazen-ter-furazanes”, Fizika Goreniya i Vzryva, 56:3 (2020), 61–68; Combustion, Explosion and Shock Waves, 56:3 (2020), 301–307
Citation in format AMSBIB
\Bibitem{LemKazSan20}
\by D.~B.~Lempert, A.~I.~Kazakov, V.~S.~Sannikov, A.~V.~Nabatova, D.~V.~Dashko, A.~I.~Stepanov
\paper Thermochemical and energy characteristics of symmetric nitro and azido derivatives of diazen-ter-furazanes
\jour Fizika Goreniya i Vzryva
\yr 2020
\vol 56
\issue 3
\pages 61--68
\mathnet{http://mi.mathnet.ru/fgv679}
\crossref{https://doi.org/10.15372/FGV20200306}
\elib{https://elibrary.ru/item.asp?id=43102279}
\transl
\jour Combustion, Explosion and Shock Waves
\yr 2020
\vol 56
\issue 3
\pages 301--307
\crossref{https://doi.org/10.1134/S0010508220030065}
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