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Fizika Goreniya i Vzryva, 2017, Volume 53, Issue 4, Pages 23–33
DOI: https://doi.org/10.15372/FGV20170402 (Mi fgv422) 		 
This article is cited in 8 scientific papers (total in 8 papers)

Experimental and numerical investigation of the chemical reaction kinetics in syngas H$_2$/ÑO flame at a pressure of 1–10 atm

D. A. Knyaz'kovab, T. A. Bolshovaa, A. M. Dmitrievac, A. G. Shmakovac, O. P. Korobeinicheva

a Voevodsky Institute of Chemical Kinetics and Combustion, Siberian Branch, Russian Academy of Sciences, Novosibirsk, 630090, Russia
b Far Eastern Federal University, Vladivostok, 690950, Russia
c Novosibirsk State University, Novosibirsk, 630090, Russia
Full-text PDF (284 kB) Citations (8)
DOI: https://doi.org/10.15372/FGV20170402
Abstract: The structure of a premixed flame of syngas (H$_2$/CO/O$_2$/Ar = 0.0667/0.0667/0.0667/0.8) stabilized on a flat burner at a pressure of 5 atm was studied experimentally and by numerical simulation. The mole fraction profiles of the reactants (Í$_2$, ÑÎ, and Î$_2$) and the major (Í$_2$Î and ÑÎ$_2$) and intermediate (Î, ÎÍ, ÍÎ$_2$, and Í$_2$Î$_2$) combustion products were measured by molecular beam mass spectrometry. The experimental data were compared with those calculated using three detailed chemical-kinetic mechanisms proposed in the literature for oxidation of a Í$_2$/ÑÎ mixture. Good agreement was found between the results of the experiment and simulation. Calculations of the structure of the flame of the same composition at a pressure of 1 and 10 atm were performed to establish the effect of the pressure on the chemical reaction kinetics in the syngas flame. The results were explained by kinetic analysis of the mechanisms.
Keywords: syngas, molecular beam mass spectrometry, premixed flame, numerical simulation, high pressure.
Funding agency Grant number
Siberian Branch of Russian Academy of Sciences II.2
Ministry of Education and Science of the Russian Federation 14.Y26.31.0003
Received: 05.12.2016
English version:
Combustion, Explosion and Shock Waves, 2017, Volume 53, Issue 4, Pages 388–397
DOI: https://doi.org/10.1134/S0010508217040025
Bibliographic databases:
Document Type: Article
UDC: 536.46
Language: Russian
Citation: D. A. Knyaz'kov, T. A. Bolshova, A. M. Dmitriev, A. G. Shmakov, O. P. Korobeinichev, “Experimental and numerical investigation of the chemical reaction kinetics in syngas H$_2$/ÑO flame at a pressure of 1–10 atm”, Fizika Goreniya i Vzryva, 53:4 (2017), 23–33; Combustion, Explosion and Shock Waves, 53:4 (2017), 388–397
Citation in format AMSBIB
\Bibitem{KnyBolDmi17}
\by D.~A.~Knyaz'kov, T.~A.~Bolshova, A.~M.~Dmitriev, A.~G.~Shmakov, O.~P.~Korobeinichev
\paper Experimental and numerical investigation of the chemical reaction kinetics in syngas H$_2$/ÑO flame at a pressure of 1--10 atm
\jour Fizika Goreniya i Vzryva
\yr 2017
\vol 53
\issue 4
\pages 23--33
\mathnet{http://mi.mathnet.ru/fgv422}
\crossref{https://doi.org/10.15372/FGV20170402}
\elib{https://elibrary.ru/item.asp?id=29772331}
\transl
\jour Combustion, Explosion and Shock Waves
\yr 2017
\vol 53
\issue 4
\pages 388--397
\crossref{https://doi.org/10.1134/S0010508217040025}
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    • This publication is cited in the following 8 articles:
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